Provided in this zip file are the inputs for Machine-learned Force Field (MLFF) and their corresponding outputs. The two folders: SOAP: Contains the training performed with VASP 1-train: The training inputs (ICONST, INCAR, KPOINTS, POSCAR, POTCAR) with outputs 2-refit: Refit the force field with previously generated ML_ABN with resultand force field files (ML_FFN) 3-phonon: The MLFF phonon calculation using finite displacement method with phonopy 4-qha: The quasi-harmonic approximation calculation with phonopy to obtain C_p values 5-validation: The validation of energy and forces on 1,000 randomly generated K3C60 distortions. ACE: Contains the training performed with FLARE package combined with Quantem Espresso 1-train: The training inputs for FLARE (init.xyz, otf_train.yaml) with concised outputs 2-hyp_scan: The scan for radius cutoff (C-C pair from 3.0 to 4.9 A and C-K pairs from 3.7 to 5.6 A, both with step size of 0.1 A) The input given (offline_train.yaml) is for the optimal in the scan, along with its correspponding force field output files (*.flare) The model likelihood for all other scans are summarized in K3C60_flare_rcutscan.csv 3-phonon: The MLFF phonon calculation using finite displacement method with phonopy. PhonoLAMMPS is used for interfacing 4-validation: The validation of energy and forces on the same aforementioned 1,000 randomly generated K3C60 distortions.